スギモリ キミカズ
  杉森 公一
   所属   高等教育推進センター
   職種   教授
言語種別 英語
発行・発表の年月 2009/11
形態種別 学術論文
査読 査読あり
標題 Laser Control of Photodissociation Process in Diatomic Molecule
執筆形態 共著
掲載誌名 INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY
掲載区分国外
出版社・発行元 JOHN WILEY&SONS INC
巻・号・頁 109(14),pp.3416-3422
著者・共著者 A. Tawada, K. Sugimori, M. Sano, S. Taniguchi, H. Nagao, K. Nishikawa
概要 In this work, we first aim to realize the complete laser-induced photodissociation of the OH molecule, and then intend to control the wavepacket generated on the continuum state, i.e., to achieve the laser control of the above-threshold dissociation (ATD) spectrum. To numerically solve the Schrodinger equation, we adopt the split operator method (SOM), which conserves the norm of the state vector, and can treat both discrete and continuum states simultaneously and correctly. This photodissociation process induced by the multiphoton absorption involves the ATD spectrum due to the continuum-continuum transition by the intense electric field. First, we investigate the detailed mechanism of the complete photodissociation with the one-color laser pulse by changing the laser parameters.
DOI 10.1002/qua.22162
ISSN 00207608