スギモリ キミカズ
杉森 公一 所属 高等教育推進センター 職種 教授 |
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言語種別 | 英語 |
発行・発表の年月 | 2006/12 |
形態種別 | 学術論文 |
査読 | 査読あり |
標題 | Theoretical study of the dissociation process by multiphoton absorption in the diatomic molecule |
執筆形態 | 共著 |
掲載誌名 | INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY |
掲載区分 | 国外 |
出版社・発行元 | JOHN WILEY&SONS INC |
巻・号・頁 | 106(15),pp.3079-3086 |
担当区分 | 筆頭著者,責任著者 |
著者・共著者 | Kimikazu Sugimori, Tomoya Ito, Yusuke Takata, Kazuhiro Ichitani, Hidemi Nagao, Kiyoshi Nishikawa |
概要 | We investigate multiphoton absorption, including the dissociation process in the OH molecule by means of wavepacket dynamics. The time-development scheme is the so-called split-operator method, which conserves the norm of the state vector. The resultant wavepacket involves the information of all discrete vibrational states and the dissociative continuum state substantially, so we are able to treat all the bound-bound, the bound-continuum and the continuum-continuum transitions. The energy spectra of the system under the strong laser pulse can also be obtained by the spectrum method, where the autocorrelation function of the wavepacket under consideration is Fourier transformed. First, we discuss the field intensity dependence of the population and the competition between dissociation and absorption processes in triultiphoton processes of above-threshold dissociation (ATD). Then, we analyze the above-threshold dissociation due to the continuum-continuum transition in detail. |
DOI | 10.1002/qua.21149 |
ISSN | 00207608 |